Enhancement of transverse thermoelectric conductivity originating from stationary points in nodal line

28 Aug 2020  ·  Susumu Minami, Fumiyuki Ishii, Motoaki Hirayama, Takuya Nomoto, Takashi Koretsune, Ryotaro Arita ·

Motivated by the recent discovery of a large anomalous Nernst effect in Co$_2$MnGa, Fe$_3X$ ($X$=Al, Ga) and Co$_3$Sn$_2$S$_2$, we performed a first-principles study to clarify the origin of the enhancement of the transverse thermoelectric conductivity ($\alpha_{ij}$) in these ferromagnets. The intrinsic contribution to $\alpha_{ij}$ can be understood in terms of the Berry curvature ($\Omega$) around the Fermi level, and $\Omega$ is singularly large along nodal lines (which are gapless in the absence of the spin-orbit coupling) in the Brillouin zone. We find that not only the Weyl points but also stationary points in the energy dispersion of the nodal lines play a crucial role. The stationary points make sharp peaks in the density of states projected onto the nodal line, clearly identifying the characteristic Fermi energies at which $\alpha_{ij}$ is most dramatically enhanced. We also find that $\alpha_{ij}/T$ breaks the Mott relation and show a peculiar temperature dependence at these energies. The present results suggest that the stationary points will give us a useful guiding principle to design magnets showing a large anomalous Nernst effect.

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Materials Science Mesoscale and Nanoscale Physics