Lattice reconstruction induced multiple ultra-flat bands in twisted bilayer WSe2

11 Mar 2021  ·  En Li, Jin-Xin Hu, Xuemeng Feng, Zishu Zhou, Liheng An, Kam Tuen Law, Ning Wang, Nian Lin ·

Moir\'e superlattices in van der Waals heterostructures provide a tunable platform to study emergent properties that are absent in the natural crystal form. Twisted bilayer transition metal dichalcogenides (TB-TMDs) can host moir\'e flat bands over a wide range of twist angles. For twist angle close to 60{\deg}, it was predicted that TB-TMDs undergo a lattice reconstruction which causes the formation of ultra-flat bands. Here, by using scanning tunneling microscopy and spectroscopy, we show the emergence of multiple ultra-flat bands in twisted bilayer WSe2 when the twist angle is larger than 57{\deg}. The bandwidth, manifested as narrow tunneling conductance peaks, is estimated less than 10meV, which is only a fraction of the estimated on-site Coulomb repulsion energy. The number of these ultra-flat bands and spatial distribution of the wavefunctions match the theoretical predictions incredibly well, strongly evidencing that the observed ultra-flat bands are induced by lattice reconstruction. Our work provides a foundation for further study of the exotic correlated phases in TB-TMDs.

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Mesoscale and Nanoscale Physics